Simulation of the Sour-Compression Unit (SCU) process for CO2 purification applied to flue gases coming from oxy-combustion cement industries

Laribi, Sinda; Dubois, Lionel; Duprez, Marie-Eve; De Weireld, Guy; Thomas, Diane

doi:10.1016/j.compchemeng.2018.11.010

Article (Scientific journals)

Simulation of the Sour-Compression Unit (SCU) process for CO2 purification applied to flue gases coming from oxy-combustion cement industries

Laribi, Sinda; Dubois, Lionel; Duprez, Marie-Eve et al.

2019 • In Computers and Chemical Engineering, 121, p. 523-539

Peer Reviewed verified by ORBi

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https://hdl.handle.net/20.500.12907/12610

DOI
10.1016/j.compchemeng.2018.11.010

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Abstract :

[en] The purpose of the present work was to investigate, for a gas issued from a full oxy-fuel combustion in the cement industry, a CO2 de-SOx and de-NOx process, called 'Sour-Compression Unit' (SCU),thanks to simulations with Aspen PlusTM. An important stage necessary for the SCU modeling has been the construction of an accurate chemical mechanism. Two-column and single-column configurations have been evaluated and compared. A parametric study and a Design Of Experiments have been conducted on a single-column process to study the influence of the operating parameters on the SOx and NOx abatement ratios. As a demonstration of the effectiveness of the model, three SOx and NOx purity specifications (depending on the further applications of the CO2) were applied to the purified gas. The feature of the investigated model lies on optimizing the way to reach the purity target in order to decrease installation costs (CAPEX) and energy requirements (OPEX).

Disciplines :

Chemical engineering
Chemistry

Author, co-author :

Laribi, Sinda

Dubois, Lionel ; Université de Mons > Faculté Polytechnique > Service de Génie des Procédés chimiques et biochimiques

Duprez, Marie-Eve ; Université de Mons > Faculté Polytechnique > Service de Thermodynamique, Physique mathématiques

De Weireld, Guy ; Université de Mons > Faculté Polytechnique > Service de Thermodynamique, Physique mathématiques

Thomas, Diane ; Université de Mons > Faculté Polytechnique > Service de Génie des Procédés chimiques et biochimiques

Language :

English

Title :

Simulation of the Sour-Compression Unit (SCU) process for CO2 purification applied to flue gases coming from oxy-combustion cement industries

Publication date :

01 February 2019

Journal title :

Computers and Chemical Engineering

ISSN :

0098-1354

eISSN :

1873-4375

Publisher :

Elsevier, United Kingdom

Volume :

121

Pages :

523-539

Peer reviewed :

Peer Reviewed verified by ORBi

Research unit :

F505 - Génie des Procédés chimiques et biochimiques
F506 - Thermodynamique, Physique mathématiques

Research institute :

R200 - Institut de Recherche en Energie

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