[en] Phytochemical investigation and bioactivity evaluation of terpenoids from the Croton species were conducted. The chemical composition of C. sylvaticus was explored using chemical phytochemical screening techniques and dereplication of 13C NMR data using MixONat software (v. 1.0.1). Natural products with diverse structural features were identified in the dichloromethane extract of trunk bark. These include monoterpenoids, sesquiterpenoids, diterpenoids, triterpenoids, along with other minor metabolites, such as steroids, saponins, and fatty acids. Further purification of this extract led to the isolation of three major secondary metabolites, acetyl aleuritolic acid, caryophyllene oxide, and phytol. These secondary metabolites were reported for the first time in C. sylvaticus. The isolated compounds were structurally compared to known anticancer terpenoids previously identified in two other Congolese Croton species. Through molecular docking studies, the predicted binding affinities of the identified compounds were assessed, and possible structure-activity relationships (SAR) were proposed. Two structurally characterized receptors-the human androgen receptor (HAR, PDB ID: 1E3G) and hypoxia-inducible factor 1-alpha (HIF-1α, PDB ID: 3KCX), known for their involvement in cancer-related pathways, were used for molecular docking investigations. Among the tested compounds, 1, 2, 3, and 12 were identified as having strong-to-moderate predicted binding affinities to both protein targets, along with favorable drug-like properties according to the ADMET analysis. This investigation could justify the use of Croton plants in traditional medicine. In addition, our study highlights the potential of the Congolese Croton species as sources of bioactive secondary metabolites.
Research center :
CMMI - Centre de Recherche en Microscopie et Imagerie Médicale
Mvingu, Bienvenu Kamalandua; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo
Nsiama, Tienabe; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo
Kanga, Obed Nsemi; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo
Taba, Kalulu Muzele; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo
Kilembe, Jason Thambwe ; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo
Mputu, Jean-Noël Kanyinda ; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo ; NMR and Molecular Imaging Laboratory, General, Organic and Biomedical Chemistry Unit, University of Mons, 19 Avenue Maistriau, 7000 Mons, Belgium
Garifo, Sarah ; Université de Mons - UMONS > Faculté de Médecine, Pharmacie et Sciences Biomédicales > Service de Chimie générale, organique et biomédicale
HENOUMONT, Céline ; Université de Mons - UMONS > Faculté de Médecine et de Pharmacie > Service de Chimie générale, organique et biomédicale
Dibwe, Dya Fita ; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo ; Faculty of Health Sciences, Hokkaido University, Kita-12, Nishi-5, Kita-Ku, Sapporo 060-0812, Japan
Mbala, Blaise Mavinga; Mention Chimie et Industrie, Faculté des Sciences et Technologies, Université de Kinshasa, Kin XI, Kinshasa P.O. Box 190, Democratic Republic of the Congo
LAURENT, Sophie ; Université de Mons - UMONS > Faculté de Médecine et de Pharmacie > Service de Chimie générale, organique et biomédicale
Language :
English
Title :
Rapid Dereplication of Trunk Bark Constituents of Croton sylvaticus and Molecular Docking of Terpenoids from Three Congolese Croton Species.
Publication date :
01 May 2025
Journal title :
International Journal of Molecular Sciences
ISSN :
1661-6596
eISSN :
1422-0067
Publisher :
Multidisciplinary Digital Publishing Institute (MDPI), Switzerland
R550 - Institut des Sciences et Technologies de la Santé R100 - Institut des Biosciences
Funding text :
The authors gratefully acknowledge the in-kind support (001-DMN-2024) provided by the omic station and Food Chemistry and Biochemistry Unit, Department of Chemistry and Industry, Faculty of Science and Technology, at the University of Kinshasa, which made this research possible.
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