Superhydrophobic Aluminum Surfaces by Deposition of Micelles of Fluorinated Block Copolymers

[en] Superhydrophobic surfaces are generated by chemisorption on aluminum substrates of fluorinated block copolymers synthesized by reversible addition-fragmentation chain transfer in supercritical carbon dioxide. In an appropriate solvent, those block copolymers can form micelles with a fluorinated corona, which are grafted on the aluminum substrate thanks to the presence of carboxylic acid groups in the corona. Water contact angle and drop impact analysis were used to characterize the wettability of the films at the macroscale, and atomic force microscopy measurements provided morphological information at the micro- and nanoscale. The simple solvent casting of the polymer solution on a hydroxylated aluminum surface results in a coating with multiscale roughness, which is fully superhydrophobic over areas up to 4 cm2.

Disciplines :

Materials science & engineering
Chemistry
Physics

Author, co-author :

Desbief, Simon ; Université de Mons > Faculté des Sciences > Chimie des matériaux nouveaux

Grignard, B.

Detrembleur, Christophe

Rioboo, Romain ; Université de Mons > Faculté des Sciences > Laboratoire de Physique des Surfaces et Interfaces

Vaillant, Alexandre ; Université de Mons > Faculté des Sciences > Laboratoire de Physique des Surfaces et Interfaces

Seveno, David

Voué, Michel ; Université de Mons > Faculté des Sciences > Physique des matériaux et Optique

De Coninck, Joël ; Université de Mons > Faculté des Sciences > Service du Laboratoire de Physique des Surfaces et Interfaces

Jonas, A.M.

Jérôme, Christine

Damman, Pascal ; Université de Mons > Faculté des Sciences > Laboratoire Interfaces et Fluides Complexes

Lazzaroni, Roberto ; Université de Mons > Faculté des Sciences > Service de Chimie des matériaux nouveaux

Language :

English

Title :

Superhydrophobic Aluminum Surfaces by Deposition of Micelles of Fluorinated Block Copolymers

Publication date :

02 February 2010

Journal title :

Langmuir

ISSN :

0743-7463

Publisher :

American Chemical Society, United States - District of Columbia

Volume :

Issue :

Pages :

2057-2067

Peer reviewed :

Peer Reviewed verified by ORBi

Research unit :

S817 - Chimie des matériaux nouveaux
S877 - Laboratoire de Physique des Surfaces et Interfaces
S885 - Laboratoire Interfaces et Fluides complexes
S878 - Physique des matériaux et Optique

Research institute :

R400 - Institut de Recherche en Science et Ingénierie des Matériaux
R150 - Institut de Recherche sur les Systèmes Complexes

Commentary :

Publié en ligne le 18 septembre 2009

Available on ORBi UMONS :

since 10 June 2010

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